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Supramolecular assembly of pyrene-DNA conjugates: influence of pyrene substitution pattern and implications for artificial LHCs.

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cris.virtual.author-orcid0000-0003-1842-9975
cris.virtual.author-orcid0000-0002-6212-2295
cris.virtual.author-orcid0000-0001-7725-5579
cris.virtual.author-orcid0000-0001-5014-4318
cris.virtualsource.author-orcid2e976d75-ec17-46aa-84fc-d7737d3226b0
cris.virtualsource.author-orcid6b67a730-db0d-4f6b-99b4-731d7b4e0d67
cris.virtualsource.author-orciddd3192fa-2c79-48e8-8703-7ae4724d6319
cris.virtualsource.author-orcid9e32d116-847d-4776-8027-b224174541e0
cris.virtualsource.author-orcide050e437-7048-4ed7-8f07-6eaad53734c2
cris.virtualsource.author-orcid287951a8-fab6-4464-b187-db7044358092
datacite.rightsopen.access
dc.contributor.authorThiede, Jan
dc.contributor.authorRothenbühler, Simon
dc.contributor.authorIacovache, Mircea Ioan
dc.contributor.authorLangenegger, Simon Matthias
dc.contributor.authorZuber, Benoît
dc.contributor.authorHäner, Robert
dc.date.accessioned2024-10-25T18:11:34Z
dc.date.available2024-10-25T18:11:34Z
dc.date.issued2023-10-11
dc.description.abstractThe supramolecular self-assembly of pyrene-DNA conjugates into nanostructures is presented. DNA functionalized with different types of pyrene isomers at the 3'-end self-assemble into nano-objects. The shape of the nanostructures is influenced by the type of pyrene isomer appended to the DNA. Multilamellar vesicles are observed with the 1,6- and 1,8-isomers, whereas conjugates of the 2,7-isomer exclusively assemble into spherical nanoparticles. Self-assembled nano-spheres obtained with the 2,7-dialkynyl pyrene isomer were used for the construction of an artificial light-harvesting complex (LHC) in combination with Cy3 as the energy acceptor.
dc.description.numberOfPages5
dc.description.sponsorshipDCBP Gruppe Prof. Häner
dc.description.sponsorshipDepartement für Chemie, Biochemie und Pharmazie (DCBP) Universität Bern
dc.description.sponsorshipInstitut für Anatomie
dc.identifier.doi10.48350/186630
dc.identifier.pmid37750811
dc.identifier.publisherDOI10.1039/d3ob01375h
dc.identifier.urihttps://boris-portal.unibe.ch/handle/20.500.12422/170242
dc.language.isoen
dc.publisherRoyal Society of Chemistry
dc.relation.ispartofOrganic & biomolecular chemistry
dc.relation.issn1477-0520
dc.relation.organization5EBDFFD4994748B4B44FD17D5E463CFB
dc.relation.organizationDCD5A442BCD7E17DE0405C82790C4DE2
dc.relation.organizationDCD5A442C14DE17DE0405C82790C4DE2
dc.subject.ddc500 - Science::570 - Life sciences; biology
dc.subject.ddc500 - Science::540 - Chemistry
dc.subject.ddc600 - Technology::610 - Medicine & health
dc.titleSupramolecular assembly of pyrene-DNA conjugates: influence of pyrene substitution pattern and implications for artificial LHCs.
dc.typearticle
dspace.entity.typePublication
dspace.file.typetext
oaire.citation.endPage7912
oaire.citation.issue39
oaire.citation.startPage7908
oaire.citation.volume21
oairecerif.author.affiliationDCBP Gruppe Prof. Häner
oairecerif.author.affiliationDepartement für Chemie, Biochemie und Pharmazie (DCBP) Universität Bern
oairecerif.author.affiliationInstitut für Anatomie
oairecerif.author.affiliationDepartement für Chemie, Biochemie und Pharmazie (DCBP) Universität Bern
oairecerif.author.affiliationInstitut für Anatomie
oairecerif.author.affiliationDepartement für Chemie, Biochemie und Pharmazie (DCBP) Universität Bern
oairecerif.author.affiliation2Departement für Chemie, Biochemie und Pharmazie (DCBP) Universität Bern
unibe.contributor.rolecreator
unibe.contributor.rolecreator
unibe.contributor.rolecreator
unibe.contributor.rolecreator
unibe.contributor.rolecreator
unibe.contributor.rolecreator
unibe.date.licenseChanged2023-09-28 15:33:05
unibe.description.ispublishedpub
unibe.eprints.legacyId186630
unibe.journal.abbrevTitleORG BIOMOL CHEM
unibe.refereedtrue
unibe.subtype.articlejournal

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